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载体组成对负载型PtSn/ZSM-5催化剂上丙烷脱氢反应性能的影响
用微型催化反应装置结合吡啶吸附的红外光谱、 NH3-程序升温脱附、热重、 H2化学吸附和程序升温还原等物理化学手段研究了载体组成对负载型PtSn/ZSM-5催化剂上丙烷脱氢反应性能的影响.结果表明,负载型PtSn/ZSM-5催化剂对丙烷脱氢的催化性能与载体组成密切相关.随着ZSM-5载体中SiO2/Al2O3比的增加,催化剂表面的酸中心总量和强酸中心量逐渐减少.当SiO2/Al2O3摩尔比从45增至108时,催化剂对丙烷脱氢反应的催化活性提高,并且催化剂的积炭量下降.当SiO2/Al2O3摩尔比增至304时, Sn组分与载体ZSM-5之间的相互作用减弱,经H2还原后催化剂中Sn0物种所占的比例增加,导致催化剂H2化学吸附量和丙烷脱氢反应活性下降.
QIU Anding
FAN Yining
作者单位：
南京大学化学化工学院,介观化学教育部重点实验室,江苏省纳米技术重点实验室,江苏南京,210093
ISTICSCIPKU
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Urethanes Technology
Urga Mitteilungen
Use of Minerals in Papermaking
User Modelling and User-Adapted Interaction
Uspekhi Fizicheskikh Nauk
Uspekhi Khimii
Vakuum in Forschung und Praxis
Valmet Paper News
VDE Fachberichte
VDI Berichte
Vector (Electrical Engineering)
Vehicle System Dynamics
Veitsch-Radex Rundschau
Verhutet Unfalle
Verpackungs - Rundschau
Vertiflite
Very Large Data Bases, International Conference Proceedings
Vesti Akademii Nauk Belorussii/News of Belorussian Academy of Sciences
Vestnik Moskovskogo Universita, Seriya 3: Fizika Astronomiya
Vestnik Moskovskogo Universiteta, Seriya 1 (Matematika Mekhanika)
Vestnik Moskovskogo Universiteta, Seriya 15: Matematika i Kibernetika
Vestnik RAN
Vestnik Rentgenologii i Radiologii
Vestnik Sankt-Peterburgskogo Universiteta. Ser 1. Matematika. Mekhanik
a. Astronomiya.
VGB PowerTech
Vibrational Spectroscopy
Vide: Science, Technique et Applications
Vision - Conference Proceedings
Vision Tecnologica
Visual Computer
VLSI Design
Volcanology and Seismology
Vom Wasser
Voprosy Izobretatel'stva
VTI Rapport
VTT Julkaisuja
VTT Symposium (Valtion Teknillinen Tutkimuskeskus)
VTT Tiedotteita - Valtion Teknillinen Tutkimuskeskus
Vysokochistye Veshchestva
Vysokomolekularnye Soedineniya. Seriya A
Vysokomolekulyarnye Soedineniya Seriya B
Walden's Fiber and Board Report
Walden's Paper Report
Waste Disposal and Water Management in Australia
Waste Management
Waste Management & Research
Water & Environment International
Water & Wastes DigeST
Water & Wastewater International
Water Environment and Technology
Water Environment Research
Water Quality International
Water Quality Research Journal of Canada
Water Research
Water Resources IMPACT
Water Resources Management
Water Resources Planning and Management: Saving a Threatened Resource
- In Search of Solutions, Proceedings of the Water Resources Sessions
at Water Forum
Water Resources Research
Water Resources Research Institute News of the University of North Carolina
Water S.A.
Water Science and Technology
Water Services
Water Supply
Water Treatment
Water Well Journal
Water, Air and Soil Pollution
Water/Engineering and Management
Watermarks
WaterWorld
Wave Motion
Waves Random Media
Wear of Materials: International Conference on Wear of Materials
Weather and Forecasting
Web Offset The Hard Copy
Weidianzixue yu Jisuanji/Microelectronics & Computer
Weixi Jiagong Jishu/Microfabrication Technology
Welding and Metal Fabrication
Welding and Surfacing Reviews
Welding Design & Fabrication
Welding in the World, Le Soudage Dans Le Monde
Welding Innovation Quarterly
Welding International
Welding Journal (Miami, Fla)
Welding Research Abroad
Welding Research Council Bulletin
Welding Research Council, Progress Reports
Welding Review International
Werkstatt und Betrieb
Werkstoffe und Korrosion
Wescon Conference Record
Western Journal of Applied Forestry
Wind & Structures, An International Journal
Wind Engineering
Winter Annual Meeting of the American Society of Mechanical Engineers
Winter School of Theoretical Physics
Winter Simulation Conference Proceedings
Wire Industry
Wire Journal International
Wireless Networks
Wireless Personal Communications
Wirtschaftsinformatik
Wissenschaftlinche Zeitschrift der Technischen Universitat Dresden
WLB Wasser, Luft und Boden
Wochenblatt fuer Papierfabrikation
Wood and Fiber Science
Wood Markets Quarterly
Wood Science and Technology
Wood Technology
Workboat Magazine
Workshop on Computer Science Logic
Workshop on Dynamics of FirST
Workshop on Fermion Algorithms
Workshop on High Performance Electron Devices for Microwave and Optoel
ectronic Applications, EDMO
Workshop on High Temperature Superconductivity
Workshop on Modern Aspects of Protein Adsorption on Biomaterials
Workshop Proceedings - Geographic Database Management Systems
World Cement
World Conference of the Textile Institute, Proceedings
World Congress on Superconductivity
World Mining Congress
World Patent Information
World Pumps
World Tunnelling and Subsurface Excavation
World Wastes
Wuhan Cehui Keji Daxue Xuebao/Journal of Wuhan Technical University of
Surveying and Mapping
Wuhan Daxue Xuebao/Journal of Wuhan University
Wuhan Gangtie Xueyuan Xuebao/Journal of Wuhan Iron and Steel University
Wuhan Gongye Daxue Xuebao/Journal of Wuhan University of Technology
Wuhan Jiaotong Keji Daxue Xuebao/Journal of Wuhan Transportation University
Wuhan Shuili Dianli Daxue Xuebao/Journal of Wuhan University of Hydrau
lic and Electric Engineering
Wuhan University Journal of Natural Sciences
Wuji Cailiao Xuebao/Journal of Inorganic Materials
Wuli Xuebao/Acta Physica Sinica
Xi Tong Gong Cheng Yu Dian Zi Ji Shu/Systems Engineering & Electronics
Xi'an Dianzi Keji Daxue Xuebao/Journal of Xidian University
Xi'an Gonglu Xueyuan Xuebao/Journal of Xi'an Highway Transportation University
Xi'an Jianzhu Keji Daxue Xuebao/Journal of Xi'an University of Archite
cture & Technology
Xi'an Shiyou Xueyuan Xuebao/Journal of Xi'an Petroleum Institute (Natu
ral Science Edition)
Xiangtan Daxue Ziran Kexue Xuebao/ Natural Science Journal of Xiangtan
University
Xiangtan Kuangye Xueyuan Xuebao/Journal of Xiangtan Mining Institute
Xiaoxing Weixing Jisuanji Xitong/Mini-Micro Systems
Xibei Gongye Daxue Xuebao/Journal of Northwestern Polytechnical University
Xinan Jiaotong Daxue Xuebao/Journal of SouthweST
Xinan Shiyou Xueyuan Xuebao/Journal of Southwestern Petroleum Institute
Xinjianzhu/New Architecture
Xinxing Jianzhu Cailiao/New Building Materials
Xitong Fangzhen Xuebao/Acta Simulata Systematica Sinica
Xitong Gongcheng Lilun yu Shijian/System Engineering Theory and Practice
Xiyou Jinshu Cailiao Yu Gongcheng/Rare Metal Materials and Engineering
X-Ray Spectrometry
Yadian Yu Shengguang/Piezoelectrics and Acoustooptics
Yanshilixue Yu Gongcheng Xuebao/Chinese Journal of Rock Mechanics and
Engineering
Yantu Gongcheng Xuebao/Chinese Journal of Geotechnical Engineering
Yejin Fenxi/Metallurgical Analysis
Yi Qi Yi Biao Xue Bao/Chinese Journal of Scientific Instrument
Yibiao Jishu Yu Chuanganqi/Instrument Technique and Sensor
Ying Yong Li Xue Xue Bao/Chinese Journal of Applied Mechanics
Yingyong Jiguang/Applied Laser Technology
Yosetsu Gakkai Ronbunshu/Quarterly Journal of the Japan Welding Society
Yosetsu Gakkai Shi/Journal of the Japan Welding Society
You Qi Chu Yun/Oil & Gas Storage and Transportation
Yuanzineng Kexue Jishu/Atomic Energy Science and Technology
Yugoslav Journal of Operations Research
Yuhang Xuebao/Journal of Astronautics
Yukagaku/Chemical Technology
Yuki Gosei Kagaku Kyokaishi/Journal of Synthetic Organic Chemistry
Zairyo to Kankyo/ Corrosion Engineering
Zairyo/Journal of the Society of Materials Science, Japan
Zashchita Metallov
Zavodskaya Laboratoriya
Zbornik Radova Pomorskog Fakulteta
Zeitschrift fuer Angewandte Mathematik und Mechanik, ZAMM, Applied Mat
hematics and Mechanics
Zeitschrift fuer Anorganische und Allgemeine Chemie
Zeitschrift fuer Auslaendische Landwirtschaft
Zeitschrift fuer Geologische Wissenschaften
Zeitschrift fuer Kristallographie
Zeitschrift fuer Metallkunde/Materials Research and Advanced Techniques
Zeitschrift fuer Naturforschung. B, Journal of Chemical Sciences
Zeitschrift fuer Naturforschung. Section A: Physical Sciences
Zeitschrift fuer Physikalische Chemie
Zeszyty Naukowe Politechniki Lodzkiej Mechanika
Zeszyty Naukowe. Geodezja
Zeszyty Naukowe. Geologia. Akademia Gorniczo-Hutnicza im. Stanislawa Staszica.
Zeszyty Naukowe. Zagadnienia Techniczno-Ekonomiczne. Akademia Gorniczo
-Hutnicza im.Stanislawa Staszica / Technical and Economical Problems
ZEV-Zeitschrift fuer Eisenbahnwesen und Verkehrstechnik - Journal for
Railway and Transport
Zhejiang Daxue Xuebao (Ziran Kexue Ban)/Journal of Zhejiang University
(Natural Science Edition)
Zhejiang Nongye Daxue Xuebao/Journal of the Zhejiang Agricultural University
Zhendong Ceshi Yu Zhenduan/Journal of Vibration, Measurement & Diagnosis
Zhendong Gongcheng Xuebao/Journal of Vibration Engineering
Zhengzhou Daxue Xuebao/Journal of Zhengzhou University
Zhenkong Kexue yu Jishu Xuebao/Vacuum Science and Technology
Zhizao Jishu Yu Jichuang/Manufacturing Technology & Machine Tool
Zhongguo Dianji Gongcheng Xuebao/Proceedings of the Chinese Society of
Electrical Engineering
Zhongguo Dianli/Electric Power
Zhongguo Gonglu Xuebao/China Journal of Highway and Transport
Zhongguo Huanjing Kexue/China Environmental Science
Zhongguo Jiguang/Chinese Journal of Lasers
Zhongguo Jishui Paishui/China Water & Wastewater
Zhongguo Jixie Gongcheng/China Mechanical Engineering
Zhongguo Kuangye Daxue Xuebao/Journal of China University of Mining &
Technology
Zhongguo Shengwu Yixue Gongcheng Xuebao/Chinese Journal of Biomedical
Engineering
Zhongguo Yaoxue Zazhi/Chinese Pharmaceutical Journal
Zhongguo Youse Jinshu Xuebao/Chinese Journal of Nonferrous Metals
Zhongguo Zaozh Xuebao/Transactions of China Pulp & Paper
Zhonghua Yixue Yichuanxue Zazhi/Chinese Journal of Medical Genetics
Zhongnan Gongye Daxue Xuebao/Journal of Central South University of Technology
Zhongshan Daxue Xuebao/Acta Scientiarum Natralium Universitatis Sunyatseni
Zhongxing Jixie/Heavy Machinery
Zhoucheng/Bearing
Zhurnal Analiticheskoi Khimii
Zhurnal Eksperimental'noi i Teoreticheskoi Fiziki
Zhurnal Neorganicheskoj Khimii
Zhurnal Obshchei Khimii
Zhurnal Prikladnoi Mekhaniki i Tekhnicheskoi Fiziki
Zhurnal Tekhnicheskoi Fiziki
Zhuzao Jishu/Foundry Technology
Zhuzao/Foundry
ZI, Ziegelindustrie International/Brick and Tile Industry International
Zidonghua Xuebao/Acta Automatica Sinica
ZKG International
ZWF Zeitschrift fuer Wirtschaftlichen Fabrikbetrieb
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